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Identifying groundwater degradation sources in a Mediterranean coastal area experiencing significant multi-origin stresses

Boumaiza Lamine, Chesnaux Romain, Drias Tarek, Walter Julien, Huneau Frédéric, Garel Emilie, Knoeller Kay et Stumpp Christine. (2020). Identifying groundwater degradation sources in a Mediterranean coastal area experiencing significant multi-origin stresses. Science of The Total Environment, 746, (141203),

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URL officielle: http://dx.doi.org/doi:10.1016/j.scitotenv.2020.141...

Résumé

This study investigates the multiple contamination sources of a coastal Mediterranean aquifer in northeastern Algeria that is bordered by two rivers and neighboring densely populated areas. Hydrogeochemical and isotopic groundwater characterization is carried out, including the analyses of major elements, water stable isotopes δ2H-H2O and δ18O-H2O, and stable isotopes of nitrate δ15N-NO3 and δ18O-NO3, and then integrated into the history of land use over the study area. Groundwater nitrate concentrations ranging from 1.6 to 235 mg/L with a median value of 69 mg/L are evidence of the degradation of groundwater quality induced by anthropogenic sources. The combined of δ15N-NO3 and δ18O-NO3 ratios showed that nitrate in groundwater is attributable to (i) the uncontrolled development of inadequate private sanitation systems over the study area, and (ii) the unsafe application of animal manure to fertilize crops. Very active saltwater intrusion is confirmed by several hydrogeochemical indicators. Interestingly, the intrusion mechanism appears to be more complex than a direct intrusion from the Mediterranean Sea. During the high-water period, saltwater intrusion may also originate from the two rivers bordering the aquifer, via upstream migration of seawater through the river mouths. The heavier ratios in δ2H-H2O and δ18O-H2O of surface water collected from the rivers suggest that water from the Mediterranean Sea is mixing with water in the rivers. Multi-source contamination not only contributes to complex chemical reactions within the aquifer, but also contributes, via the cumulative effect of the various sources, to affecting large parts of the study area. The present study may serve as a warning to the effect that historical land-use practices may exert seriously deleterious impacts on groundwater quality and greatly limit conditions for the sustainable management of Mediterranean coastal areas.

Type de document:Article publié dans une revue avec comité d'évaluation
Volume:746
Numéro:141203
Version évaluée par les pairs:Oui
Date:Décembre 2020
Sujets:Sciences naturelles et génie > Génie
Sciences naturelles et génie > Sciences appliquées
Sciences naturelles et génie > Sciences naturelles > Sciences de la terre (géologie, géographie)
Département, module, service et unité de recherche:Départements et modules > Département des sciences appliquées > Unité d'enseignement en sciences de la Terre
Mots-clés:Aquifer, stable isotopes, nitrate, seawater intrusion, groundwater contamination, hydrogeochemistry, North Africa, aquifère, isotopes stables, nitrate, intrusion d'eau de mer, contamination des eaux souterraines, hydrogéochimie, Afrique du Nord
Déposé le:01 sept. 2020 23:22
Dernière modification:01 sept. 2020 23:22
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